Paper
Breakdown of the isotropic asymptotic approximation in two-colour photoionisation
Authors
Sooraj Rajendran, Miguel Benito de Lama, Praveen Kumar Maroju, Michele Di Fraia, Oksana Plekan, David Busto, Ioannis Makos, Marvin Schmoll, Luca Giannessi, Enrico Allaria, Primož Rebernik Ribič, Giovanni De Ninno, Alexander Demidovich, Miltcho Danailov, Marco Zangrando, Kenneth J. Schafer, Richard J. Squibb, Raimund Feifel, Tamás Csizmadia, Fabio Frassetto, Luca Poletto, Kevin C. Prince, Johan Mauritsson, Carlo Callegari, Johannes Feist, Alicia Palacios, Giuseppe Sansone
Abstract
The Wigner delay is defined as the energy derivative of the scattering phase of a particle in a given potential, unveiling the time taken (or gained) due to the interaction. The characterisation of this delay plays a central role in attosecond science, where the time resolution allows to gain information on the time interval required for a photoelectron to be emitted into the continuum after the absorption of a single photon. Attosecond interferometric techniques, based on two-colour (extreme ultraviolet and near-infrared) photoionisation schemes, cannot provide a direct measurement of the Wigner delay, because the low-frequency photon contributes with an additional delay, which is imprinted on the outgoing photoelectron. The isolation of the Wigner delay is usually achieved by appealing to the asymptotic approximation, which assumes that the two-photon delay is separable into a Wigner and a near-infrared-induced phase and provides a universal analytical expression for the latter. In this study, we introduce a self-referencing approach based on the implementation of non-consecutive extreme ultraviolet harmonics, in order to test the validity of the asymptotic approximation. We demonstrate its breakdown by observing a deviation of a few tens of milliradians (corresponding to a few attoseconds) between its predictions and the experimentally measured phases of the sideband oscillations generated in our scheme, in agreement with full-dimensional simulations.
Metadata
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Raw Data (Debug)
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"raw_xml": "<entry>\n <id>http://arxiv.org/abs/2603.15293v1</id>\n <title>Breakdown of the isotropic asymptotic approximation in two-colour photoionisation</title>\n <updated>2026-03-16T13:55:08Z</updated>\n <link href='https://arxiv.org/abs/2603.15293v1' rel='alternate' type='text/html'/>\n <link href='https://arxiv.org/pdf/2603.15293v1' rel='related' title='pdf' type='application/pdf'/>\n <summary>The Wigner delay is defined as the energy derivative of the scattering phase of a particle in a given potential, unveiling the time taken (or gained) due to the interaction. The characterisation of this delay plays a central role in attosecond science, where the time resolution allows to gain information on the time interval required for a photoelectron to be emitted into the continuum after the absorption of a single photon. Attosecond interferometric techniques, based on two-colour (extreme ultraviolet and near-infrared) photoionisation schemes, cannot provide a direct measurement of the Wigner delay, because the low-frequency photon contributes with an additional delay, which is imprinted on the outgoing photoelectron. The isolation of the Wigner delay is usually achieved by appealing to the asymptotic approximation, which assumes that the two-photon delay is separable into a Wigner and a near-infrared-induced phase and provides a universal analytical expression for the latter.\n In this study, we introduce a self-referencing approach based on the implementation of non-consecutive extreme ultraviolet harmonics, in order to test the validity of the asymptotic approximation. We demonstrate its breakdown by observing a deviation of a few tens of milliradians (corresponding to a few attoseconds) between its predictions and the experimentally measured phases of the sideband oscillations generated in our scheme, in agreement with full-dimensional simulations.</summary>\n <category scheme='http://arxiv.org/schemas/atom' term='physics.atom-ph'/>\n <published>2026-03-16T13:55:08Z</published>\n <arxiv:primary_category term='physics.atom-ph'/>\n <author>\n <name>Sooraj Rajendran</name>\n </author>\n <author>\n <name>Miguel Benito de Lama</name>\n </author>\n <author>\n <name>Praveen Kumar Maroju</name>\n </author>\n <author>\n <name>Michele Di Fraia</name>\n </author>\n <author>\n <name>Oksana Plekan</name>\n </author>\n <author>\n <name>David Busto</name>\n </author>\n <author>\n <name>Ioannis Makos</name>\n </author>\n <author>\n <name>Marvin Schmoll</name>\n </author>\n <author>\n <name>Luca Giannessi</name>\n </author>\n <author>\n <name>Enrico Allaria</name>\n </author>\n <author>\n <name>Primož Rebernik Ribič</name>\n </author>\n <author>\n <name>Giovanni De Ninno</name>\n </author>\n <author>\n <name>Alexander Demidovich</name>\n </author>\n <author>\n <name>Miltcho Danailov</name>\n </author>\n <author>\n <name>Marco Zangrando</name>\n </author>\n <author>\n <name>Kenneth J. Schafer</name>\n </author>\n <author>\n <name>Richard J. Squibb</name>\n </author>\n <author>\n <name>Raimund Feifel</name>\n </author>\n <author>\n <name>Tamás Csizmadia</name>\n </author>\n <author>\n <name>Fabio Frassetto</name>\n </author>\n <author>\n <name>Luca Poletto</name>\n </author>\n <author>\n <name>Kevin C. Prince</name>\n </author>\n <author>\n <name>Johan Mauritsson</name>\n </author>\n <author>\n <name>Carlo Callegari</name>\n </author>\n <author>\n <name>Johannes Feist</name>\n </author>\n <author>\n <name>Alicia Palacios</name>\n </author>\n <author>\n <name>Giuseppe Sansone</name>\n </author>\n </entry>"
}